Bart will play an employee at the hotel in Farhampton where Barney (Harris) and Robin (Cobie Smulders) will get married this season.
The series, which will return for its final season Sept. 23, also features Alyson Hannigan, Josh Radnor and Jason Segel.
Bart, who took home the Tony Award in 1999 for his performance in You're a Good Man, Charlie Brown, was Tony-nominated for his performance in The Producers and has also been seen in The Frogs, Triumph of Love, King David and Big River.
Sheria Irving and Gabriel Ebert lead the company of the Public Theater production.
Matthew Gardiner is directing the '60s rock musical at the D.C.-area theatre.
The stars showed up in Art Deco-inspired looks and many shades of green for the new musical about artist Tamara de Lempicka.
Plus, Dylan Mulvaney, J. Harrison Ghee, Sara Bareilles, and other stars walked the red carpet.
The season, opening September 21, will include 58 ballets across 21 weeks of performances.
The evening will mark the 30th anniversary of the original animated film while also celebrating its long-running stage musical adaptation.
Gordon Greenberg will direct the revised musical version of the Oscar-nominated Ang Lee film.
Due to the expansive nature of Off-Broadway, this list is not comprehensive.
Gabriel Vick is continuing his performance as Daniel Hillard as the London run of the musical enters its second year.
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